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Model-based Interpretation of the Performance and Degradation of Reformate Fueled Solid Oxide Fuel Cells

Model-based Interpretation of the Performance and Degradation of Reformate Fueled Solid Oxide Fuel Cells

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Solid oxide fuel cells offer great prospects for the sustainable, clean and safe conversion of various fuels into electrical energy. In this thesis, the performance-determining loss processes for the cell operation on reformate fuels are elucidated via electrochemical impedance spectroscopy. Model-based analyses reveal the electrochemical fuel oxidation mechanism, the coupling of fuel gas transport and reforming chemistry and the impact of fuel impurities on the degradation of each loss process.

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Keywords

  • electrochemistry
  • impedance spectroscopy
  • modeling
  • Reforming Chemistry
  • SOFC

Links

DOI: 10.5445/KSP/1000034160

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